General approach for \$m\$ bits
The general solution for a test for division by 3 is to sum up the even-numbered bits and separately sum up the odd-numbered bits, take the difference between these sums, and then see if the difference itself is divisible by 3. (There are a variety of approaches for this operation, but the one encountered first is usually via carry-save adders.)
For a binary value with \$m\$ bits, where \$m\$ is even, the difference will require at most \$\lceil\operatorname{ln}_2\frac{m}{2}\rceil\$ bits. For a binary value with \$m\$ bits, where \$m\$ is odd, the difference will require at most \$\lceil\operatorname{ln}_2\frac{m+1}{2}\rceil\$ bits. This difference result could itself then be submitted to a much smaller tier for, once again, computing the difference between the sums of even and odd numbered bits. (And repeat.)
Specific case where \$m=4\$
At this point it is pretty easy to see that the even and odd sums can be computed using a simple half-adder, each. The resulting table is:
$$
\begin{smallmatrix}\begin{array}{r|cccc}
&\overline{C_\text{odd}}\:\overline{S_\text{odd}}&\overline{C_\text{odd}}\:S_\text{odd}&C_\text{odd}\:\overline{S_\text{odd}}\\
\hline
\overline{C_\text{even}}\:\overline{S_\text{even}}&Y&N&N\\
\overline{C_\text{even}}\:S_\text{even}&N&Y&N\\
C_\text{even}\:\overline{S_\text{even}}&N&N&Y
\end{array}\end{smallmatrix}
$$
In this case, there is no need to worry about "divisibility by 3" of the difference. Instead, it's sufficient to compare the two sums for "equal," as shown in the above table.
This should be very easy to implement:
simulate this circuit – Schematic created using CircuitLab
The half-adders are easily recognized above. In addition, their associated outputs are directly compared using a pair of XORs. The results of these two comparisons are then considered using a NOR for the final output.